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- Disc 1
- 1I Am a Rock2:41
- 2Leaves That Are Green2:30
- 3A Church Is Burning3:23
- 4April Come She Will1:47
- 5The Sound of Silence3:06
- 6A Most Peculiar Man2:23
- 7He Was My Brother2:46
- 8Kathy's Song3:28
- 9The Side of a Hill2:17
- 10A Simple Desultory Philippic (Or How I Was Robert McNamara'd Into Submission)2:17
- 11Flowers Never Bend with the Rainfall2:17
- 12Patterns3:03
- 13I Am a Rock (Alternate Version)2:44
- 14A Church Is Burning (Alternate Version)3:10
- Disc 2
- 1Mother and Child Reunion3:07
- 2Duncan4:43
- 3Everything Put Together Falls Apart2:01
- 4Run That Body Down3:52
- 5Armistice Day3:55
- 6Me and Julio Down by the Schoolyard2:44
- 7Peace Like a River3:23
- 8Papa Hobo2:35
- 9Hobo's Blues1:20
- 10Paranoia Blues2:56
- 11Congratulations3:43
- 12Me and Julio Down by the Schoolyard (Demo - San Francisco 2/71)2:27
- 13Duncan (Demo - San Francisco 2/71)2:46
- 14Paranoia Blues (Unreleased Version)3:14
- Disc 3
- 1Kodachrome3:35
- 2Tenderness2:55
- 3Take Me to the Mardi Gras3:30
- 4Something so Right4:36
- 5One Man's Ceiling Is Another Man's Floor3:47
- 6American Tune3:45
- 7Was a Sunny Day3:44
- 8Learn How to Fall2:47
- 9St. Judy's Comet3:21
- 10Loves Me Like a Rock3:33
- 11Let Me Live In Your City (Work In Progress)4:20
- 12Take Me to the Mardi Gras (Acoustic Demo)2:29
- 13American Tune (Unfinished Demo)4:01
- 14Loves Me Like a Rock (Acoustic Demo)3:24
- Disc 4
- 1Me and Julio Down by the Schoolyard (with The Jessy Dixon Singers & Urubamba) [Live 1973]2:47
- 2Homeward Bound (with The Jessy Dixon Singers & Urubamba) [Live 1973]2:44
- 3American Tune (with The Jessy Dixon Singers & Urubamba) [Live 1973]4:01
- 4El Condor Pasa (If I Could) [with The Jessy Dixon Singers & Urubamba] [Live 1973]4:05
- 5Duncan (with The Jessy Dixon Singers & Urubamba) [Live 1973]5:07
- 6The Boxer (with The Jessy Dixon Singers & Urubamba) [Live 1973]6:07
- 7Mother and Child Reunion (with The Jessy Dixon Singers & Urubamba) [Live 1973]4:02
- 8The Sound of Silence (with The Jessy Dixon Singers & Urubamba) [Live 1973]4:24
- 9Jesus Is the Answer (with The Jessy Dixon Singers & Urubamba) [Live 1973]3:26
- 10Bridge over Troubled Water (with The Jessy Dixon Singers & Urubamba) [Live 1973]7:28
- 11Loves Me Like a Rock (with The Jessy Dixon Singers & Urubamba) [Live 1973]3:01
- 12America (with The Jessy Dixon Singers & Urubamba) [Live 1973]4:33
- 13Kodachrome (Live 1973)2:55
- 14Something so Right (Live 1973)4:34
- Disc 5
- 1Still Crazy After All These Years3:26
- 2My Little Town (with Art Garfunkel)3:51
- 3I Do It for Your Love3:35
- 450 Ways to Leave Your Lover3:37
- 5Night Game2:57
- 6Gone at Last (with Phoebe Snow & The Jessy Dixon Singers)3:40
- 7Some Folks' Lives Roll Easy3:14
- 8Have a Good Time3:26
- 9You're Kind3:20
- 10Silent Eyes4:05
- 11Slip Slidin' Away (Demo)5:29
- 12Gone at Last (Original Demo with The Jessy Dixon Singers)4:38
- Disc 6
- 1Late in the Evening4:02
- 2That's Why God Made the Movies3:37
- 3One-Trick Pony (Live at the Agora Theatre, Cleveland, OH - September 1979)3:53
- 4How the Heart Approaches What It Yearns2:49
- 5Oh, Marion4:00
- 6Ace in the Hole (Live at the Agora Theatre, Cleveland, OH - September 1979)5:43
- 7Nobody3:32
- 8Jonah3:30
- 9God Bless the Absentee3:17
- 10Long, Long Day3:50
- 11Soft Parachutes (Unreleased Soundtrack Recording)1:51
- 12All Because of You (Outtake)4:05
- 13Spiral Highway (Unreleased Soundtrack Recording)2:55
- 14Stranded in a Limosine3:10
- Disc 7
- 1Allergies4:39
- 2Hearts and Bones5:39
- 3When Numbers Get Serious3:26
- 4Think Too Much (b)2:45
- 5Song About the Moon4:11
- 6Think Too Much (a)3:05
- 7Train in the Distance5:12
- 8Rene and Georgette Magritte with Their Dog After the War3:43
- 9Cars Are Cars3:15
- 10The Late Great Johnny Ace4:47
- 11Shelter of Your Arms (Unreleased Work-In-Progress)3:09
- 12Train in the Distance (Original Acoustic Demo)3:11
- 13Rene and Georgette Magritte with Their Dog After the War (Original Acoustic Demo)3:45
- 14The Late Great Johnny Ace (Original Acoustic Demo)3:22
- Disc 8
- 1The Boy In the Bubble3:59
- 2Graceland4:51
- 3I Know What I Know (with General M.D.Shirinda & The Gaza Sisters)3:13
- 4Gumboots (with Boyoyo Boys)2:44
- 5Diamonds on the Soles of Her Shoes5:49
- 6You Can Call Me Al4:40
- 7Under African Skies3:37
- 8Homeless (with Ladysmith Black Mambazo)3:48
- 9Crazy Love, Vol. II4:19
- 10That Was Your Mother (with Rockin' Dopsie & The Twisters)2:52
- 11All Around the World or the Myth of Fingerprints (with Los Lobos)3:16
- 12Homeless (Demo)2:30
- 13Diamonds on the Soles of Her Shoes (Alternate Unreleased Version)4:41
- 14All Around the World or the Myth of Fingerprints (Early Version) [Early Version]3:17
- 15You Can Call Me Al (Demo)2:04
- 16Crazy Love (Demo)2:31
- 17The Story of "Graceland" as Told by Paul Simon9:38
- Disc 9
- 1The Obvious Child4:10
- 2Can't Run But3:36
- 3The Coast5:04
- 4Proof4:39
- 5Further to Fly5:36
- 6She Moves On5:03
- 7Born at the Right Time3:48
- 8The Cool, Cool River4:33
- 9Spirit Voices3:56
- 10The Rhythm of the Saints4:12
- 11Born at the Right Time (Original Acoustic Demo) [Bonus Track]3:50
- 12Thelma (Bonus Track)4:14
- 13The Coast (Work-In-Progress) [Bonus Track]5:13
- 14Spirit Voices (Work-In-Progress) [Bonus Track]3:49
- Disc 10
- 1The Obvious Child (Live at Central Park, New York, NY - August 15, 1991)4:38
- 2The Boy in the Bubble (Live at Central Park, New York, NY - August 15, 1991)5:59
- 3She Moves On (Live at Central Park, New York, NY - August 15, 1991)6:26
- 4Kodachrome (Live at Central Park, New York, NY - August 15, 1991)4:13
- 5Born at the Right Time (Live at Central Park, New York, NY - August 15, 1991)5:11
- 6Train in the Distance (Live at Central Park, New York, NY - August 15, 1991)4:45
- 7Me and Julio Down by the Schoolyard (Live at Central Park, New York, NY - August 15, 1991)3:14
- 8I Know What I Know (Live at Central Park, New York, NY - August 15, 1991)4:45
- 9The Cool, Cool River (Live at Central Park, New York, NY - August 15, 1991)5:41
- 10Bridge over Troubled Water (Live at Central Park, New York, NY - August 15, 1991)5:16
- 11Proof (Live at Central Park, New York, NY - August 15, 1991)5:40
- Disc 11
- 1The Coast (Live at Central Park, New York, NY - August 15, 1991)7:06
- 2Graceland (Live at Central Park, New York, NY - August 15, 1991)5:31
- 3You Can Call Me Al (Live at Central Park, New York, NY - August 15, 1991)5:10
- 4Still Crazy After All These Years (Live at Central Park, New York, NY - August 15, 1991)3:42
- 5Loves Me Like a Rock (Live at Central Park, New York, NY - August 15, 1991)2:54
- 6Diamonds on the Soles of Her Shoes (Live at Central Park, New York, NY - August 15, 1991)9:31
- 7Hearts and Bones (Live at Central Park, New York, NY - August 15, 1991)6:18
- 8Late in the Evening (Live at Central Park, New York, NY - August 15, 1991)4:45
- 9America (Live at Central Park, New York, NY - August 15, 1991)3:23
- 10The Boxer (Live at Central Park, New York, NY - August 15, 1991)4:18
- 11Cecilia (Live at Central Park, New York, NY - August 15, 1991)3:24
- 12The Sound of Silence (Live at Central Park, New York, NY - August 15, 1991)5:46
- Disc 12
- 1Adios Hermanos4:42
- 2Born in Puerto Rico4:54
- 3Satin Summer Nights5:45
- 4Bernadette3:28
- 5The Vampires5:05
- 6Quality4:10
- 7Can I Forgive Him6:02
- 8Sunday Afternoon3:25
- 9Killer Wants to Go to College1:51
- 10Time Is an Ocean5:23
- 11Virgil2:49
- 12Killer Wants to Go to College II2:09
- 13Trailways Bus5:15
- 14Shoplifting Clothes (Bonus Track)3:35
- 15Born in Puerto Rico (Demo with Jose Feliciano) [Bonus Track]4:59
- 16Can I Forgive Him (Original Demo) [Bonus Track]1:56
- Disc 13
- 1That's Where I Belong3:12
- 2Darling Lorraine6:38
- 3Old2:19
- 4You're the One4:27
- 5The Teacher3:36
- 6Look at That3:54
- 7Señorita with a Necklace of Tears3:41
- 8Love3:50
- 9Pigs, Sheep and Wolves3:58
- 10Hurricane Eye4:11
- 11Quiet4:17
- 12That's Where I Belong (Live)3:42
- 13Old (Live)2:40
- 14Hurricane Eye (Live)6:00
- Disc 14
- 1How Can You Live in the Northeast?3:42
- 2Everything About It Is a Love Song3:57
- 3Outrageous3:24
- 4Sure Don't Feel Like Love3:57
- 5Wartime Prayers4:49
- 6Beautiful3:07
- 7I Don't Believe4:09
- 8Another Galaxy5:22
- 9Once Upon a Time There Was an Ocean3:55
- 10That's Me4:43
- 11Father and Daughter4:11
- Disc 15
- 1Getting Ready for Christmas Day4:06
- 2The Afterlife3:40
- 3Dazzling Blue4:32
- 4Rewrite3:49
- 5Love and Hard Times4:09
- 6Love Is Eternal Sacred Light4:02
- 7Amulet1:36
- 8Question for the Angels3:49
- 9Love & Blessings4:18